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Size-controllable synthesis of monodispersed nitrogen-doped carbon nanospheres from polydopamine forhigh-rate supercapacitors

《化学科学与工程前沿（英文）》 2023年 第17卷 第11期   页码 1788-1800 doi: 10.1007/s11705-023-2326-8

摘要： Monodispersed nitrogen-doped carbon nanospheres with tunable particle size (100–230 nm) were synthesized via self-polymerization of biochemical dopamine in the presence of hexamethylenetetramine as a buffer and F127 as a size controlling agent. Hexamethylenetetramine can mildly release NH3, which in turn initiates the polymerization reaction of dopamine. The carbon nanospheres obtained exhibited a significant energy storage capability of 265 F·g–1 at 0.5 A·g–1 and high-rate performance of 82% in 6 mol·L–1 KOH (20 A·g–1), which could be attributed to the presence of abundant micro-mesoporous structure, doped nitrogen functional groups and the small particle size. Moreover, the fabricated symmetric supercapacitor device displayed a high stability of 94% after 5000 cycles, revealing the considerable potential of carbon nanospheres as electrode materials for energy storage.

关键词： carbon nanospheres     size-controlled     nitrogen-doped     high-rate     supercapacitors    

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SUSTAINABLE NITROGEN MANAGEMENT FOR VEGETABLE PRODUCTION IN CHINA

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 373-385 doi: 10.15302/J-FASE-2022455

摘要：

● Sustainable nitrogen management strategies for Chinese vegetable production are summarized.

关键词： enhanced-efficiency nitrogen fertilizer     integrated knowledge and products strategy     nitrogen rate     reactive nitrogen loss     vegetable     yield    

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REGIONAL ASSESSMENT OF SOIL NITROGEN MINERALIZATION IN DIVERSE CROPLAND OF A REPRESENTATIVE INTENSIVE

《农业科学与工程前沿（英文）》 2023年 第10卷 第4期   页码 530-540 doi: 10.15302/J-FASE-2023515

摘要：

Soil nitrogen mineralization (Nmin) is a key process that converts organic N into mineral N that controls soil N availability to plants. However, regional assessments of soil Nmin in cropland and its affecting factors are lacking, especially in relation to variation in elevation. In this study, a 4-week incubation experiment was implemented to measure net soil Nmin rate, gross nitrification (Nit) rate and corresponding soil abiotic properties in five field soils (A–C, maize; D, flue-cured tobacco; and E, vegetables; with elevation decreasing from A to E) from different altitudes in a typical intensive agricultural area in Dali City, Yunnan Province, China. The results showed that soil Nmin rate ranged from 0.10 to 0.17 mg·kg−1·d−1 N, with the highest value observed in field E, followed by fields D, C, B, and A, which indicated that soil Nmin and Nit rates varied between fields, decreasing with elevation. The soil Nit rate ranged from 434.2 to 827.1 µg·kg−1·h−1 N, with the highest value determined in field D, followed by those in fields E, C, B, and A. The rates of soil Nmin and Nit were positively correlated with several key soil parameters, including total soil N, dissolved organic carbon and dissolved inorganic N across all fields, which indicated that soil variables regulated soil Nmin and Nit in cropland fields. In addition, a strong positive relationship was observed between soil Nmin and Nit. These findings provide a greater understanding of the response of soil Nmin among cropland fields related to spatial variation. It is suggested that the soil Nmin from cropland should be considered in the evaluation of the N transformations at the regional scale.

关键词： cropland     gross nitrification rate     regulatory factors     soil nitrogen mineralization     spatial variation    

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Reconsideration on the effect of nitrogen on mixed culture polyhydroxyalkanoate production toward high

Zhiqiang Chen, Lizhi Zhao, Ye Ji, Qinxue Wen, Long Huang

《环境科学与工程前沿（英文）》 2019年 第13卷 第4期 doi: 10.1007/s11783-019-1135-2

摘要：

Effect of nitrogen on mixed culture PHA production was reconsidered.

Enrichment history of PHA accumulating culture was discussed.

Higher PHA content and biomass growth were achieved in presence of nitrogen.

Enrichment strategy toward higher PHA accumulation was investigated.

Microbial community succession in PHA accumulation phase was investigated.

关键词： Polyhydroxyalkanoate (PHA)     Organic loading rate     Nitrogen content     Biomass growth     Enrichment history    

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An integrated approach to site-specific management zone delineation

Yuxin MIAO, David J. MULLA, Pierre C. ROBERT

《农业科学与工程前沿（英文）》 2018年 第5卷 第4期   页码 432-441 doi: 10.15302/J-FASE-2018230

摘要：

Dividing fields into a few relatively homogeneous management zones (MZ) is a practical and cost-effective approach to precision agriculture. There are three basic approaches to MZ delineation using soil and/or landscape properties, yield information, and both sources of information. The objective of this study is to propose an integrated approach to delineating site-specific MZ using relative elevation, organic matter, slope, electrical conductivity, yield spatial trend map, and yield temporal stability map (ROSE-YSTTS) and evaluate it against two other approaches using only soil and landscape information (ROSE) or clustering multiple year yield maps (CMYYM). The study was carried out on two no-till corn-soybean rotation fields in eastern Illinois, USA. Two years of nitrogen (N) rate experiments were conducted in Field B to evaluate the delineated MZs for site-specific N management. It was found that in general the ROSE approach was least effective in accounting for crop yield variability (8.0%–9.8%), while the CMYYM approach was least effective in accounting for soil and landscape (8.9%–38.1%), and soil nutrient and pH variability (9.4%–14.5%). The integrated ROSE-YSTTS approach was reasonably effective in accounting for the three sources of variability (38.6%–48.9%, 16.1%–17.3% and 13.2%–18.7% for soil and landscape, nutrient and pH, and yield variability, respectively), being either the best or second best approach. It was also found that the ROSE-YSTTS approach was effective in defining zones with high, medium and low economically optimum N rates. It is concluded that the integrated ROSE-YSTTS approach combining soil, landscape and yield spatial-temporal variability information can overcome the weaknesses of approaches using only soil, landscape or yield information, and is more robust for MZ delineation. It also has the potential for site-specific N management for improved economic returns. More studies are needed to further evaluate their appropriateness for precision N and crop management.

关键词： economically optimum nitrogen rate     fuzzy cluster analysis     precision nitrogen management     site-specific management     soil landscape property     yield map    

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SUSTAINABLE NITROGEN MANAGEMENT IN AUSTRALIAN AGROECOSYSTEMS: CHALLENGES AND OPPORTUNITIES

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 366-372 doi: 10.15302/J-FASE-2022447

摘要：

● There is huge potential for improvement of nitrogen management in Australia.

关键词： Australian agroecosystems     reactive nitrogen     sustainable development    

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EFFECTS OF SUBSTITUTION OF MINERAL NITROGEN WITH ORGANIC AMENDMENTS ON NITROGEN LOSS FROM SLOPING CROPLAND

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 396-406 doi: 10.15302/J-FASE-2022456

摘要：

● Interflow acts as the dominant pathway for N loss loadings.

关键词： improved fertilization regime     interflow     nitrogen forms     nitrogen leaching     purple soil     sloping cropland    

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Nitrogen distribution in the products from the hydrothermal liquefaction of sp. and sp.

《化学科学与工程前沿（英文）》 2022年 第16卷 第6期   页码 985-995 doi: 10.1007/s11705-021-2126-y

摘要： The high contents of nitrogen-containing organic compounds in biocrude obtained from hydrothermal liquefaction of microalgae are one of the most concerned issues on the applications and environment. In the project, Chlorella sp. and Spirulina sp. were selected as raw materials to investigate the influence of different reaction conditions (i.e., reaction temperature, residence time, solid loading rate) on the distribution of nitrogen in the oil phase and aqueous phase. Three main forms of nitrogen-containing organic compounds including nitrogen-heterocyclic compounds, amide, and amine were detected in biocrudes. The contents of nitrogen-heterocyclic compounds decreased with temperature while amide kept increasing. The effect of residence time on the components of nitrogen-containing organic compounds was similar with that of temperature. However, the influence of solid loading rate was insignificant. Moreover, it was also found that the differences of amino acids in the protein components in the two microalgae might affect the nitrogen distribution in products. For example, nitrogen in basic amino acids of Spirulina sp. preferred to go into the aqueous phase comparing with the nitrogen in neutral amino acids of Chlorella sp. In summary, a brief reaction map was proposed to describe the nitrogen pathway during microalgae hydrothermal liquefaction.

关键词： microalgae     hydrothermal liquefaction     biocrude     nitrogen distribution    

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SOIL NITROGEN CYCLING AND ENVIRONMENTAL IMPACTS IN THE SUBTROPICAL HILLY REGION OF CHINA: EVIDENCE FROM

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 407-424 doi: 10.15302/J-FASE-2022448

摘要：

● Soil nitrogen fluxes and influencing factors were reviewed in the subtropical hilly regions.

关键词： nitrogen cycling     soil nitrogen     nitrogen deposition     greenhouse gases emission     non-point source pollution     nitrogen use efficiency    

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PROGRESS ON IMPROVING AGRICULTURAL NITROGEN USE EFFICIENCY: UK-CHINA VIRTUAL JOINT CENTERS ON NITROGEN

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 475-489 doi: 10.15302/J-FASE-2022459

摘要：

● Virtual joint centers on N agronomy were established between UK and China.

关键词： CINAg     N-CIRCLE     nitrogen use efficiency     reactive nitrogen     sustainable production    

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IMPROVING NITROGEN SAFETY IN CHINA: NITROGEN FLOWS, POLLUTION AND CONTROL

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 465-474 doi: 10.15302/J-FASE-2022454

摘要：

● It is necessary to address the N flows and their impacts on environment in China for sustainable N management.

关键词： barriers     future management     ammonia emissions     nitrogen input     water N pollution    

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The combined effects of biomass and temperature on maximum specific ammonia oxidation rate in domestic

《环境科学与工程前沿（英文）》 2021年 第15卷 第6期 doi: 10.1007/s11783-021-1411-9

摘要：

• Actual SAORs was determined using MLVSS and temperature.

关键词： Specific ammonia oxidation rate     Sequencing batch reactor     Biomass     Temperature coefficient     Model simulation    

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Recent advances and challenges of nitrogen/nitrate electro catalytic reduction to ammonia synthesis

《能源前沿（英文）》 doi: 10.1007/s11708-023-0908-2

摘要： The Haber-Bosch process is the most widely used synthetic ammonia technology at present. Since its invention, it has provided an important guarantee for global food security. However, the traditional Haber-Bosch ammonia synthesis process consumes a lot of energy and causes serious environmental pollution. Under the serious pressure of energy and environment, a green, clean, and sustainable ammonia synthesis route is urgently needed. Electrochemical synthesis of ammonia is a green and mild new method for preparing ammonia, which can directly convert nitrogen or nitrate into ammonia using electricity driven by solar, wind, or water energy, without greenhouse gas and toxic gas emissions. Herein, the basic mechanism of the nitrogen reduction reaction (NRR) to ammonia and nitrate reduction reaction (NO3− RR) to ammonia were discussed. The representative approaches and major technologies, such as lithium mediated electrolysis and solid oxide electrolysis cell (SOEC) electrolysis for NRR, high activity catalyst and advanced electrochemical device fabrication for NO3 − RR and electrochemical ammonia synthesis were summarized. Based on the above discussion and analysis, the main challenges and development directions for electrochemical ammonia synthesis were further proposed.

关键词： electrochemical ammonia synthesis     nitrogen     nitrate     nitrogen reduction reaction (NRR) to ammonia     nitrate reduction reaction (NO–3 RR)    

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Use of float consumption rate in resource leveling of construction projects

Atilla DAMCI, Gul POLAT, Firat Dogu AKIN, Harun TURKOGLU

《工程管理前沿（英文）》 2022年 第9卷 第1期   页码 135-147 doi: 10.1007/s42524-020-0118-0

摘要： The management of resources has been claimed to be as important as scheduling methods. Inefficiency in managing resources may bring about severe delays and cost overruns caused by resource shortages in some cases and/or idle resources in others. Therefore, resources should be utilized efficiently to prevent project failures. Resource leveling is one of the approaches that are used for the management of resources. It aims to minimize fluctuations, peaks, and valleys in resource utilization without changing the completion time of a project and the number of resources required. Although the main principle behind traditional resource leveling is achieving an even flow of resources while the original project duration remains unchanged, the literature supports the need to develop an efficient model that discriminates among the activities that are selected for participation in resource leveling. For this purpose, this study has developed a model that considers the float consumption rates of activities in resource leveling. The float consumption rate is the percentage that is set to determine the maximum amount of float which will be consumed to shift the start time of the activity. The proposed model allows a scheduler to assign float consumption rates to each activity that can be used during the resource leveling procedure. When the required information is inputted, the proposed model automatically changes the required daily resources as it shifts the noncritical activities along their available total float times. The proposed model is expected to minimize the likelihood of severe delays and cost overruns. The model is demonstrated by constructing a network and its resource utilization histograms.

关键词： resource management     resource leveling     float consumption rate     scheduling    

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ECOLOGICAL EFFECTS OF NITROGEN DEPOSITION ON URBAN FORESTS: AN OVERVIEW

《农业科学与工程前沿（英文）》 2022年 第9卷 第3期   页码 445-456 doi: 10.15302/J-FASE-2021429

摘要：

● Patterns and effects of N deposition on urban forests are reviewed.

关键词： biodiversity     carbon sequestration     nitrogen deposition     nutrient imbalance     soil acidification     urban forest    

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标题 作者 时间 类型 操作

Size-controllable synthesis of monodispersed nitrogen-doped carbon nanospheres from polydopamine forhigh-rate supercapacitors

期刊论文

SUSTAINABLE NITROGEN MANAGEMENT FOR VEGETABLE PRODUCTION IN CHINA

期刊论文

REGIONAL ASSESSMENT OF SOIL NITROGEN MINERALIZATION IN DIVERSE CROPLAND OF A REPRESENTATIVE INTENSIVE

期刊论文

Reconsideration on the effect of nitrogen on mixed culture polyhydroxyalkanoate production toward high

Zhiqiang Chen, Lizhi Zhao, Ye Ji, Qinxue Wen, Long Huang

期刊论文

An integrated approach to site-specific management zone delineation

Yuxin MIAO, David J. MULLA, Pierre C. ROBERT

期刊论文

SUSTAINABLE NITROGEN MANAGEMENT IN AUSTRALIAN AGROECOSYSTEMS: CHALLENGES AND OPPORTUNITIES

期刊论文

EFFECTS OF SUBSTITUTION OF MINERAL NITROGEN WITH ORGANIC AMENDMENTS ON NITROGEN LOSS FROM SLOPING CROPLAND

期刊论文

Nitrogen distribution in the products from the hydrothermal liquefaction of sp. and sp.

期刊论文

SOIL NITROGEN CYCLING AND ENVIRONMENTAL IMPACTS IN THE SUBTROPICAL HILLY REGION OF CHINA: EVIDENCE FROM

期刊论文

PROGRESS ON IMPROVING AGRICULTURAL NITROGEN USE EFFICIENCY: UK-CHINA VIRTUAL JOINT CENTERS ON NITROGEN

期刊论文

IMPROVING NITROGEN SAFETY IN CHINA: NITROGEN FLOWS, POLLUTION AND CONTROL

期刊论文

The combined effects of biomass and temperature on maximum specific ammonia oxidation rate in domestic

期刊论文

Recent advances and challenges of nitrogen/nitrate electro catalytic reduction to ammonia synthesis

期刊论文

Use of float consumption rate in resource leveling of construction projects

Atilla DAMCI, Gul POLAT, Firat Dogu AKIN, Harun TURKOGLU

期刊论文

ECOLOGICAL EFFECTS OF NITROGEN DEPOSITION ON URBAN FORESTS: AN OVERVIEW

期刊论文